A Note on Aerosol Processing by Droplet Collision‐Coalescence

The processing of aerosol by droplet collision-coalescence is analyzed in three-dimensional simulations of drizzling stratocumulus using a Lagrangian cloud model for the representation of aerosol and cloud microphysics. Collision-coalescence processing is shown to create a characteristic bimodality in the aerosol size distribution. We show that the large-scale dynamics of the stratocumulus-topped boundary layer are key to understanding the amount of time available for collision-coalescence processing. The large-scale dynamics enable aerosol particles to repeat a cycle of droplet condensation, collision-coalescence, and evaporation, which causes a steady increase in aerosol size. This process is continued until the aerosol grows so large that droplet growth is substantially accelerated and multiple collisions occur within one cycle, forming precipitation-sized droplets that are lost to the surface, including the aerosol. An analytical relationship is derived that captures the fundamental shape of the processed aerosol size distribution

Cloud droplet growth in shallow cumulus clouds considering 1-D and 3-D thermal radiative effects

The effect of 1-D and 3-D thermal radiation on cloud droplet growth in shallow cumulus clouds is investigated using large eddy simulations with size-resolved cloud microphysics. A two-step approach is used for separating microphysical effects from dynamical feedbacks. In step one, an offline parcel model is used to describe the onset of rain. The growth of cloud droplets to raindrops is simulated with bin-resolved microphysics along previously recorded Lagrangian trajectories. It is shown that thermal heating and cooling rates can enhance droplet growth and raindrop production. Droplets grow to larger size bins in the 10-30 mu m radius range. The main effect in terms of raindrop production arises from recirculating parcels, where a small number of droplets are exposed to strong thermal cooling at cloud edge. These recirculating parcels, comprising about 6%-7% of all parcels investigated, make up 45% of the rain for the no-radiation simulation and up to 60% when 3-D radiative effects are considered. The effect of 3-D thermal radiation on rain production is stronger than that of 1-D thermal radiation. Three-dimensional thermal radiation can enhance the rain amount up to 40% compared to standard droplet growth without radiative effects in this idealized framework. In the second stage, fully coupled large eddy simulations show that dynamical effects are stronger than microphysical effects, as far as the production of rain is concerned. Three-dimensional thermal radiative effects again exceed one-dimensional thermal radiative effects. Small amounts of rain are produced in more clouds (over a larger area of the domain) when thermal radiation is applied to microphysics. The dynamical feedback is shown to be an enhanced cloud circulation with stronger subsiding shells at the cloud edges due to thermal cooling and stronger updraft velocities in the cloud center. It is shown that an evaporation-circulation feedback reduces the amount of rain produced in simulations where 3-D thermal radiation is applied to microphysics and dynamics, in comparison to where 3-D thermal radiation is only applied to dynamics

Investigation of the Aerosol Indirect Effect at the Southern Great Plains Using Ground-Based Remote Sensors and Modeling

The attached document is the final report in association with closeou

The Invigoration of Deep Convective Clouds Over the Atlantic: Aerosol Effect, Meteorology or Retrieval Artifact?

Associations between cloud properties and aerosol loading are frequently observed in products derived from satellite measurements. These observed trends between clouds and aerosol optical depth suggest aerosol modification of cloud dynamics, yet there are uncertainties involved in satellite retrievals that have the potential to lead to incorrect conclusions. Two of the most challenging problems are addressed here: the potential for retrieved aerosol optical depth to be cloud-contaminated, and as a result, artificially correlated with cloud parameters; and the potential for correlations between aerosol and cloud parameters to be erroneously considered to be causal. Here these issues are tackled directly by studying the effects of the aerosol on convective clouds in the tropical Atlantic Ocean using satellite remote sensing, a chemical transport model, and a reanalysis of meteorological fields. Results show that there is a robust positive correlation between cloud fraction or cloud top height and the aerosol optical depth, regardless of whether a stringent filtering of aerosol measurements in the vicinity of clouds is applied, or not. These same positive correlations emerge when replacing the observed aerosol field with that derived from a chemical transport model. Model-reanalysis data is used to address the causality question by providing meteorological context for the satellite observations. A correlation exercise between the full suite of meteorological fields derived from model reanalysis and satellite-derived cloud fields shows that observed cloud top height and cloud fraction correlate best with model pressure updraft velocity and relative humidity. Observed aerosol optical depth does correlate with meteorological parameters but usually different parameters from those that correlate with observed cloud fields. The result is a near-orthogonal influence of aerosol and meteorological fields on cloud top height and cloud fraction. The results strengthen the case that the aerosol does play a role in invigorating convective clouds

The Radiative Properties of Small Clouds: Multi-Scale Observations and Modeling

Warm, liquid clouds and their representation in climate models continue to represent one of the most significant unknowns in climate sensitivity and climate change. Our project combines ARM observations, LES modeling, and satellite imagery to characterize shallow clouds and the role of aerosol in modifying their radiative effects

A novel ensemble method for retrieving properties of warm cloud in 3-D using ground-based scanning radar and zenith radiances

We present a novel method for retrieving high-resolution, three-dimensional (3-D) nonprecipitating cloud fields in both overcast and broken-cloud situations. The method uses scanning cloud radar and multiwavelength zenith radiances to obtain gridded 3-D liquid water content (LWC) and effective radius (re) and 2-D column mean droplet number concentration (Nd). By using an adaption of the ensemble Kalman filter, radiances are used to constrain the optical properties of the clouds using a forward model that employs full 3-D radiative transfer while also providing full error statistics given the uncertainty in the observations. To evaluate the new method, we first perform retrievals using synthetic measurements from a challenging cumulus cloud field produced by a large-eddy simulation snapshot. Uncertainty due to measurement error in overhead clouds is estimated at 20% in LWC and 6% in re, but the true error can be greater due to uncertainties in the assumed droplet size distribution and radiative transfer. Over the entire domain, LWC and re are retrieved with average error 0.05–0.08 g m-3 and ~2 μm, respectively, depending on the number of radiance channels used. The method is then evaluated using real data from the Atmospheric Radiation Measurement program Mobile Facility at the Azores. Two case studies are considered, one stratocumulus and one cumulus. Where available, the liquid water path retrieved directly above the observation site was found to be in good agreement with independent values obtained from microwave radiometer measurements, with an error of 20 g m-2

An assessment of aerosol‐cloud interactions in marine stratus clouds based on surface remote sensing

An assessment of aerosol-cloud interactions (ACI) from ground-based remote sensing under coastal stratiform clouds is presented. The assessment utilizes a long-term, high temporal resolution data set from the Atmospheric Radiation Measurement (ARM) Program deployment at Pt. Reyes, California, United States, in 2005 to provide statistically robust measures of ACI and to characterize the variability of the measures based on variability in environmental conditions and observational approaches. The average ACIN (= dlnNd/dlna, the change in cloud drop number concentration with aerosol concentration) is 0.48, within a physically plausible range of 0–1.0. Values vary between 0.18 and 0.69 with dependence on (1) the assumption of constant cloud liquid water path (LWP), (2) the relative value of cloud LWP, (3) methods for retrieving Nd, (4) aerosol size distribution, (5) updraft velocity, and (6) the scale and resolution of observations. The sensitivity of the local, diurnally averaged radiative forcing to this variability in ACIN values, assuming an aerosol perturbation of 500 c-3 relative to a background concentration of 100 cm-3, ranges betwee-4 and -9 W -2. Further characterization of ACI and its variability is required to reduce uncertainties in global radiative forcing estimates